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Bioinspired cellulose-based membranes in oily wastewater treatment

《环境科学与工程前沿（英文）》 2022年 第16卷 第7期 doi: 10.1007/s11783-021-1515-2

摘要：

• Cellulose-based membrane separates oily wastewater mimicking the living things.

关键词： Cellulose     Bioinspired membrane     Superhydrophobic surface     Underwater superoleophobic surface     Oil-water separation    

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Comparison of CNT-PVA membrane and commercial polymeric membranes in treatment of emulsified oily wastewater

Gang Yi, Xinfei Fan, Xie Quan, Shuo Chen, Hongtao Yu

《环境科学与工程前沿（英文）》 2019年 第13卷 第2期 doi: 10.1007/s11783-019-1103-x

摘要：

CNT-PVA membrane was fabricated and compared with polymeric membranes.

The separation performance was evaluated by homemade and cutting fluid emulsions.

The three membranes show similar oil retention rates.

CNT-PVA membranes have higher permeation fluxes compared with polymeric membranes.

CNT-PVA membrane shows higher fouling resistance.

关键词： Oily wastewater     Microfiltration     Carbon nanotube membrane     Commercial polymeric membrane    

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Preparation and characterization of hydrothermally engineered TiO

Kanchapogu Suresh, G. Pugazhenthi, R. Uppaluri

《化学科学与工程前沿（英文）》 2017年 第11卷 第2期   页码 266-279 doi: 10.1007/s11705-017-1608-4

摘要： This work targets the preparation and characterization of an inexpensive TiO -fly ash composite membrane for oily wastewater treatment. The composite membrane was fabricated by depositing a hydrophilic TiO layer on a fly ash membrane via the hydrothermal method, and its structural, morphological and mechanical properties were evaluated. The separation potential of the composite membrane was evaluated for 100–200 mg·L synthetic oily wastewater solutions. The results show that the composite membrane has excellent separation performance and can provide permeate stream with oil concentration of only 0.26–5.83 mg·L . Compared with the fly ash membrane in the average permeate flux and performance index (49.97 × 10 m ·m ·s and 0.4620%, respectively), the composite membrane exhibits better performance (51.63 × 10 m ·m ·s and 0.4974%). For the composite ash membrane, the response surface methodology based analysis inferred that the optimum process parameters to achieve maximum membrane flux and rejection are 207 kPa, 200 mg·L and 0.1769 m·s for applied pressure, feed concentration and cross flow velocity, respectively. Under these conditions, predicted responses are 41.33 × 10 m ·m ·s permeate flux and 98.7% rejection, which are in good agreement with the values obtained from experimental investigations (42.84 × 10 m ·m ·s and 98.82%). Therefore, we have demonstrated that the TiO -fly ash composite membrane as value added product is an efficient way to recycle fly ash and thus mitigate environmental hazards associated with the disposal of oily wastewaters.

关键词： TiO2-fly ash membrane     oily wastewater     fouling     microfiltration    

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Chemical reactions of oily sludge catalyzed by iron oxide under supercritical water gasification condition

《化学科学与工程前沿（英文）》 2022年 第16卷 第6期   页码 886-896 doi: 10.1007/s11705-021-2125-z

摘要： Supercritical water gasification is a promising technology in dealing with the degradation of hazardous waste, such as oily sludge, accompanied by the production of fuel gases. To evaluate the mechanism of Fe2O3 catalyst and the migration pathways of heteroatoms and to investigate the systems during the process, reactive force field molecular dynamics simulations are adopted. In terms of the catalytic mechanisms of Fe2O3, the surface lattice oxygen is consumed by small carbon fragments to produce CO and CO2, improving the catalytic performance of the cluster due to more unsaturated coordination Fe sites exposed. Lattice oxygen combines with •H radicals to form water molecules, improving the catalytic performance. Furthermore, the pathway of asphaltene degradation was revealed at an atomic level, as well as products. Moreover, the adsorption of hydroxyl radical on the S atom caused breakage of the two C–S bonds in turn, forming •HSO intermediate, so that the organic S element was fixed into the inorganic liquid phase. The heteroatom O was removed under the effects of supercritical water. Heavy metal particles presented in the oily sludge, such as iron in association with Fe2O3 catalyst, helped accelerate the degradation of asphaltenes.

关键词： oily sludge     SCWG     ReaxFF     Fe2O3     heteroatoms    

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Occurrence and migration of microplastics and plasticizers in different wastewater and sludge treatmentunits in municipal wastewater treatment plant

《环境科学与工程前沿（英文）》 2022年 第16卷 第11期 doi: 10.1007/s11783-022-1577-9

摘要：

● Reduce the quantifying MPs time by using Nile red staining.

关键词： Microplastics     Municipal wastewater treatment plant     Phthalate esters     Thermal hydrolysis    

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Microplastics in municipal wastewater treatment plants: a case study of Denizli/Turkey

《环境科学与工程前沿（英文）》 2023年 第17卷 第8期 doi: 10.1007/s11783-023-1699-8

摘要：

● High amounts of microplastics are released to receiving media from WWTPs.

关键词： Microplastics     Wastewater treatment plant     Removal efficiency     Daily discharge    

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Membrane bioreactors for hospital wastewater treatment: recent advancements in membranes and processes

《化学科学与工程前沿（英文）》 2022年 第16卷 第5期   页码 634-660 doi: 10.1007/s11705-021-2107-1

摘要： Discharged hospital wastewater contains various pathogenic microorganisms, antibiotic groups, toxic organic compounds, radioactive elements, and ionic pollutants. These contaminants harm the environment and human health causing the spread of disease. Thus, effective treatment of hospital wastewater is an urgent task for sustainable development. Membranes, with controllable porous and nonporous structures, have been rapidly developed for molecular separations. In particular, membrane bioreactor (MBR) technology demonstrated high removal efficiency toward organic compounds and low waste sludge production. To further enhance the separation efficiency and achieve material recovery from hospital waste streams, novel concepts of MBRs and their applications are rapidly evolved through hybridizing novel membranes (non hydrophilic ultrafiltration/microfiltration) into the MBR units (hybrid MBRs) or the MBR as a pretreatment step and integrating other membrane processes as subsequent secondary purification step (integrated MBR-membrane systems). However, there is a lack of reviews on the latest advancement in MBR technologies for hospital wastewater treatment, and analysis on its major challenges and future trends. This review started with an overview of main pollutants in common hospital wastewater, followed by an understanding on the key performance indicators/criteria in MBR membranes (i.e., solute selectivity) and processes (e.g., fouling). Then, an in-depth analysis was provided into the recent development of hybrid MBR and integrated MBR-membrane system concepts, and applications correlated with wastewater sources, with a particular focus on hospital wastewaters. It is anticipated that this review will shed light on the knowledge gaps in the field, highlighting the potential contribution of hybrid MBRs and integrated MBR-membrane systems toward global epidemic prevention.

关键词： membrane technology     membrane bioreactor     hospital wastewater     hybrid MBR     integrated MBR-membrane system    

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Co-pyrolysis of oil sludge with hydrogen-rich plastics in a vertical stirring reactor: Kinetic analysis, emissions, and products

《环境科学与工程前沿（英文）》 2022年 第16卷 第10期 doi: 10.1007/s11783-022-1570-3

摘要：

● Collaborative treatment of plastics and OS was established to improve oil quality.

关键词： Oily sludge     Pyrolysis     Polyethylene     H/Ceff ratio     Oil quality    

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China Launched the First Wastewater Resource Recovery Factory in Yixing

《环境科学与工程前沿（英文）》 2022年 第16卷 第1期 doi: 10.1007/s11783-021-1496-1

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Inhibition character of crotonaldehyde manufacture wastewater on biological acidification

《环境科学与工程前沿（英文）》 2021年 第15卷 第6期 doi: 10.1007/s11783-021-1403-9

摘要：

• The inhibition of the main organic pollutions in CMW was demonstrated.

关键词： Crotonaldehyde manufacture wastewater     Biological acidification     Volatile fatty acids     Inhibition     Toxic units    

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“NEW” resource recovery from wastewater using bioelectrochemical systems: Moving forward with functions

Akshay Jain, Zhen He

《环境科学与工程前沿（英文）》 2018年 第12卷 第4期 doi: 10.1007/s11783-018-1052-9

摘要：

Resource recovery from wastewater is a key function of bioelectrochemical systems.

NEW resources to recover include Nutrient, Energy, and Water.

Identifying proper application niches can guide BES research and development.

More efforts should be invested to the application of recovered resources.

A mindset for energy performance and system scaling is critically important.

关键词： Bioelectrochemical systems     Resource recovery     Wastewater treatment     Energy     Nutrients    

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Recent progress in electrospun nanofibers and their applications in heavy metal wastewater treatment

《化学科学与工程前沿（英文）》 2023年 第17卷 第3期   页码 249-275 doi: 10.1007/s11705-022-2245-0

摘要： Novel adsorbents with a simple preparation process and large capacity for removing highly toxic and nondegradable heavy metals from water have drawn the attention of researchers. Electrospun nanofiber membranes usually have the advantages of large specific surface areas and high porosity and allowing flexible control and easy functionalization. These membranes show remarkable application potential in the field of heavy metal wastewater treatment. In this paper, the electrospinning technologies, process types, and the structures and types of nanofibers that can be prepared are reviewed, and the relationships among process, structure and properties are discussed. On one hand, based on the different components of electrospun nanofibers, the use of organic, inorganic and organic−inorganic nanofiber membrane adsorbents in heavy metal wastewater treatment are introduced, and their advantages and future development are summarized and prospected. On the other hand, based on the microstructure and overall structure of the nanofiber membrane, the recent progresses of electrospun functional membranes for heavy metal removal are reviewed, and the advantages of different structures for applications are concluded. Overall, this study lays the foundation for future research aiming to provide more novel structured adsorbents.

关键词： electrospinning     heavy metal     adsorption     nanostructure     wastewater    

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Photosensitivity sources of dissolved organic matter from wastewater treatment plants and their mediation

《环境科学与工程前沿（英文）》 2023年 第17卷 第6期 doi: 10.1007/s11783-023-1669-1

摘要：

● EE2 photodegradation behavior in the presence of four WWTPs’ DOM was explored.

关键词： Photosensitivity sources     17α-ethinylestradiol     Photodegradation     Dissolved organic matter     Wastewater treatment plants    

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Construction of defect-containing UiO-66/MoSe heterojunctions with superior photocatalytic performance for wastewater

《化学科学与工程前沿（英文）》 2023年 第17卷 第4期   页码 449-459 doi: 10.1007/s11705-022-2226-3

摘要： Metal–organic frameworks are recognized as promising multifunctional materials, especially metal–organic framework-based photocatalysts, which are considered to be ideal photocatalytic materials. Herein, a new type of UiO-66/MoSe2 composite was prepared using the solvothermal method. The optimum composite was selected by adjusting the mass ratio of UiO-66 and MoSe2. X-ray diffraction analysis showed that the mass ratio influenced the crystal plane exposure rate of the composite, which may have affected its photocatalytic performance. The composite is composed of ultra-thin flower-like MoSe2 that wrapped around cubic UiO-66, a structure that increases the abundance of active sites for reactions and is more conducive to the separation of carriers. The photocatalytic properties of the composite were evaluated by measuring the degradation rate of Rhodamine B and the catalyst’s ability to reduce Cr(VI)-containing wastewater under visible light irradiation. Rhodamine B was decolorized completely in 120 min, and most of the Cr(VI) was reduced within 150 min. The photochemical mechanism of the complex was studied in detail. The existence of Mo6+ and oxygen vacancies, in addition to the Z-type heterojunction promote the separation of electrons and holes, which enhances the photocatalytic effect.

关键词： UiO-66/MoSe2     photocatalysis     dye-containing wastewater     heavy metal wastewater     oxygen vacancies    

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Submerged arc plasma system combined with ozone oxidation for the treatment of wastewater containing

《环境科学与工程前沿（英文）》 2021年 第15卷 第5期 doi: 10.1007/s11783-020-1384-0

摘要：

• Submerged arc plasma was introduced in terms of wastewater treatment.

关键词： Thermal plasma     Submerged arc plasma     Wastewater     Ozone     Phenol     Highly energetic electron    

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标题 作者 时间 类型 操作

Bioinspired cellulose-based membranes in oily wastewater treatment

期刊论文

Comparison of CNT-PVA membrane and commercial polymeric membranes in treatment of emulsified oily wastewater

Gang Yi, Xinfei Fan, Xie Quan, Shuo Chen, Hongtao Yu

期刊论文

Preparation and characterization of hydrothermally engineered TiO

Kanchapogu Suresh, G. Pugazhenthi, R. Uppaluri

期刊论文

Chemical reactions of oily sludge catalyzed by iron oxide under supercritical water gasification condition

期刊论文

Occurrence and migration of microplastics and plasticizers in different wastewater and sludge treatmentunits in municipal wastewater treatment plant

期刊论文

Microplastics in municipal wastewater treatment plants: a case study of Denizli/Turkey

期刊论文

Membrane bioreactors for hospital wastewater treatment: recent advancements in membranes and processes

期刊论文

Co-pyrolysis of oil sludge with hydrogen-rich plastics in a vertical stirring reactor: Kinetic analysis, emissions, and products

期刊论文

China Launched the First Wastewater Resource Recovery Factory in Yixing

期刊论文

Inhibition character of crotonaldehyde manufacture wastewater on biological acidification

期刊论文

“NEW” resource recovery from wastewater using bioelectrochemical systems: Moving forward with functions

Akshay Jain, Zhen He

期刊论文

Recent progress in electrospun nanofibers and their applications in heavy metal wastewater treatment

期刊论文

Photosensitivity sources of dissolved organic matter from wastewater treatment plants and their mediation

期刊论文

Construction of defect-containing UiO-66/MoSe heterojunctions with superior photocatalytic performance for wastewater

期刊论文

Submerged arc plasma system combined with ozone oxidation for the treatment of wastewater containing

期刊论文